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New article: Bacterial-cellulose, self-adhesive sweat sensors for eco-friendly health monitoring

Pushing bacterial cellulose into a transformative product for wearable sensor applications! Our biosynthesised nanocellulose is used here for the first time as a substrate enabling the screen printing of electrochemical sensors for real-time, non-invasive alcohol monitoring in sweat. The bacterial cellulose sweat alcohol sensor has a highly linear response to alcohol concentration in human sweat, with a minimum detection concentration of 5mM and excellent reproducibility. In addition to sustainability, it shows excellent biocompatibility and self-adhesion. The sensor’s bidirectional functionality also opens new avenues for innovative sweat-sensing system designs.

Eco-Friendly Conformal and Self-Adhesive Electrochemical Sensors for Sweat Monitoring is a new paper by NN researchers Xiaohe Wang, Muling Zeng, Mabel Torrens, Martí Gich, and Anna Roig. It has been published in the journal ACS Applied Materials & Interfaces. This research was done in close collaboration with Pengfei Niu (Tianjin University) and César Fernández Sánchez (IMB-CNM and CIBER-BBN).

Title

Eco-Friendly Conformal and Self-Adhesive Electrochemical Sensors for Sweat Monitoring

DOI: 10.1021/acsami.5c07032

Abstract

Wearable sweat-sensing platforms represent a transformative advancement in noninvasive, real-time health monitoring, enabling personalized healthcare. For in vivo applications, sensor substrate materials require biocompatibility, secure adhesion, and, preferably, environmental sustainability. However, existing substrate materials fail to meet some of those requirements. This study introduces bacterial cellulose (BC) as a novel sensor substrate, leveraging its printability, biocompatibility, self-adhesion, and eco-friendliness. A wearable sweat sensor was fabricated by screen-printing conductive inks onto BC films. A key challenge addressed was the hydrophilicity of BC, which can cause liquid penetration and disrupt signal stability. To solve this, an approach was developed where the electrical tracks are sandwiched between two hydrophobic layers to fully avoid liquid interference and ensure stable electrochemical performance. The sensor was further functionalized with the alcohol oxidase enzyme to enable reliable alcohol detection in sweat at the relevant concentration range. This work demonstrates the feasibility of BC-based sensors for their application in wearable health monitoring, meanwhile promoting sustainable technological innovations in personalized healthcare and well-being technologies.

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